In this work, γ-ray shielding and Cs immobilisation performances of high-density magnetite (MG) and iron powder (IP) in Portland cement (PC) based-S/S treatment were investigated. Experimental results were elaborated using a γ-radiation shielding (γRS) index-based approach for assessing the effectiveness of in situ S/S of137Cs-contaminated soils. Main results reveal that the replacement of PC by MG or IP (up to 50%) leads to a marked increase (up to about 4-fold) in the γ-ray shielding performance, whereas a further material addition decreases the S/S shielding performance. The highest γRS index of â¼26% (662 keV) was found in the case of IP addition (33.3%). The use of MG-mixes allows reaching slightly slower γRS index jointly with the highest Cs-immobilisation of 97.8%. In this case, calculation shows a maximum137Cs-contamination level successfully treatable by in situ S/S up to â¼2.9 or â¼14.5 kBq kgâ1for the realistic or low probability scenario, respectively, highlighting the possibility to remediate a very wide range of real contamination. Findings show MG - PC S/S as the best choice and could provide a basis for decision-making of S/S remediation of137Cs-contaminated sites.
Stabilisation/solidification of Cs-137-contaminated soils using novel high-density grouts: gamma-ray shielding properties, contaminant immobilisation and a gamma RS index-based approach for in situ applicability
Falciglia, Pietro P.
;Romano, Stefano;Vagliasindi, Federico
2017-01-01
Abstract
In this work, γ-ray shielding and Cs immobilisation performances of high-density magnetite (MG) and iron powder (IP) in Portland cement (PC) based-S/S treatment were investigated. Experimental results were elaborated using a γ-radiation shielding (γRS) index-based approach for assessing the effectiveness of in situ S/S of137Cs-contaminated soils. Main results reveal that the replacement of PC by MG or IP (up to 50%) leads to a marked increase (up to about 4-fold) in the γ-ray shielding performance, whereas a further material addition decreases the S/S shielding performance. The highest γRS index of â¼26% (662 keV) was found in the case of IP addition (33.3%). The use of MG-mixes allows reaching slightly slower γRS index jointly with the highest Cs-immobilisation of 97.8%. In this case, calculation shows a maximum137Cs-contamination level successfully treatable by in situ S/S up to â¼2.9 or â¼14.5 kBq kgâ1for the realistic or low probability scenario, respectively, highlighting the possibility to remediate a very wide range of real contamination. Findings show MG - PC S/S as the best choice and could provide a basis for decision-making of S/S remediation of137Cs-contaminated sites.File | Dimensione | Formato | |
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