We present a theoretical investigation of the voltage-driven metal-insulator transition based on solving coupled Boltzmann and Hartree-Fock equations to determine the insulating gap and the electron distribution in a model system: a one-dimensional charge density wave. Electric fields that are parametrically small relative to energy gaps can shift the electron distribution away from the momentum-space region where interband relaxation is efficient, leading to a highly nonequilibrium quasiparticle distribution even in the absence of Zener tunneling. The gap equation is found to have regions of multistability; a nonequilibrium analog of the free energy is constructed and used to determine which phase is preferred.

Voltage-induced metal-insulator transition in a one-dimensional charge density wave

Chiriacò, Giuliano
Primo
;
2018-01-01

Abstract

We present a theoretical investigation of the voltage-driven metal-insulator transition based on solving coupled Boltzmann and Hartree-Fock equations to determine the insulating gap and the electron distribution in a model system: a one-dimensional charge density wave. Electric fields that are parametrically small relative to energy gaps can shift the electron distribution away from the momentum-space region where interband relaxation is efficient, leading to a highly nonequilibrium quasiparticle distribution even in the absence of Zener tunneling. The gap equation is found to have regions of multistability; a nonequilibrium analog of the free energy is constructed and used to determine which phase is preferred.
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.11769/574632
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