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Background: The 14N(n, p) 14C reaction is of interest in neutron capturetherapy, where nitrogen-related dose is the main component due tolow-energy neutrons, and in astrophysics, where 14N acts as a neutronpoison in the s process. Several discrepancies remain between theexisting data obtained in partial energy ranges: thermal energy, keVregion, and resonance region. Purpose: We aim to measure the 14N(n, p)14C cross section from thermal to the resonance region in a singlemeasurement for the first time, including characterization of the firstresonances, and provide calculations of Maxwellian averaged crosssections (MACS). Method: We apply the time-of-flight technique atExperimental Area 2 (EAR-2) of the neutron time-of-flight (n\_TOF)facility at CERN. 10B(n, \& alpha;) 7Li and 235U(n, f ) reactions areused as references. Two detection systems are run simultaneously, one onbeam and another off beam. Resonances are described with the R-matrixcode SAMMY. Results: The cross section was measured from subthermalenergy to 800 keV, resolving the first two resonances (at 492.7 and 644keV). A thermal cross section was obtained (1.809 \& PLUSMN; 0.045 b)that is lower than the two most recent measurements by slightly morethan one standard deviation, but in line with the ENDF/B-VIII.0 andJEFF-3.3 evaluations. A 1/v energy dependence of the cross section wasconfirmed up to tens of keV neutron energy. The low energy tail of thefirst resonance at 492.7 keV is lower than suggested by evaluatedvalues, while the overall resonance strength agrees with evaluations.Conclusions: Our measurement has allowed determination of the 14N(n, p)cross section over a wide energy range for the first time. We haveobtained cross sections with high accuracy (2.5\%) from subthermalenergy to 800 keV and used these data to calculate the MACS for kT = 5to kT = 100 keV.
Measurement of the 14N(n, p) 14C cross section at the CERN n\_TOF
facility from subthermal energy to 800 keV
Torres-Sanchez;Pablo and Praena;Javier and Porras;Ignacio and Sabate-Gilarte;Marta and Lederer-Woods;Claudia and Aberle;Oliver and Alcayne;Victor and Amaducci;Simone and Andrzejewski;Jozef and Audouin;Laurent and Becares;Vicente and Babiano-Suarez;Victor and Bacak;Michael and Barbagallo;Massimo and Becvar;Frantisek and Bellia;Giorgio and Berthoumieux;Eric and Billowes;Jon and Bosnar;Damir and Brown;Adam and Busso;Maurizio and Caamano;Manuel and Caballero;Luis and Calvino;Francisco and Calviani;Marco and Cano-Ott;Daniel and Casanovas;Adria and Cerutti;Francesco and Chen;Yonghao and Chiaveri;Enrico and Colonna;Nicola and Cortes;Guillem and Cortes-Giraldo;Miguel and Cosentino;Luigi and Cristallo;Sergio and Damone;Lucia-Anna and Diakaki;Maria and Dietz;Mirco and Domingo-Pardo;Cesar and Dressler;Rugard and Dupont;Emmeric and Duran;Ignacio and Eleme;Zinovia and Fernandez-Dominguez;Beatriz and Ferrari;Alfredo and Ferrer;Francisco Javier and Finocchiaro;Paolo and Furman;Valter and Goebel;Kathrin and Garg;Ruchi and Gawlik-Rami;Aleksandra and Geslot;Benoit and Gilardoni;Simone and Glodariu;Tudor and Goncalves;Isabel and Gonzalez-Romero;Enrique and Guerrero;Carlos and Gunsing;Frank and Harada;Hideo and Heinitz;Stephan and Heyse;Jan and Jenkins;David and Jericha;Erwin and Kappeler;Franz and Kadi;Yacine and Kimura;Atsushi and Kivel;Niko and Kokkoris;Michael and Kopatch;Yury and Krticka;Milan and Kurtulgil;Deniz and Ladarescu;Ion and Leeb;Helmut and Lerendegui-Marco;Jorge and Lo Meo;Sergio and Lonsdale;Sarah-Jane and Macina;Daniela and Manna;Alice and Martinez;Trinitario and Masi;Alessandro and Massimi;Cristian and Mastinu;Pierfrancesco and Mastromarco;Mario and Matteucci;Francesca and Maugeri;Emilio-Andrea and Mazzone;Annamaria and Mendoza;Emilio and Mengoni;Alberto and Michalopoulou;Veatriki and Milazzo;Paolo Maria and Mingrone;Federica and;Musumarra Agatino;and Negret;Alexandru and Nolte;Ralf and Ogallar;Francisco and Oprea;Andreea and Patronis;Nikolas and Pavlik;Andreas and Perkowski;Jaroslaw and Persanti;Luciano and Quesada;Jose-Manuel and Radeck;Desiree and Ramos-Doval;Diego and Rauscher;Thomas and Reifarth;Rene and Rochman;Dimitri and Rubbia;Carlo and Saxena;Alok and Schillebeeckx;Peter and Schumann;Dorothea and Smith;Gavin and Sosnin;Nikolay and Stamatopoulos;Athanasios and Tagliente;Giuseppe and Tain;Jose and Talip;Zeynep and Tarifeno-Saldivia;Ariel and Tassan-Got;Laurent and Tsinganis;Andrea and Ulrich;Jiri and Urlass;Sebastian and Valenta;Stanislav and Vannini;Gianni and Variale;Vincenzo and Vaz;Pedro and Ventura;Alberto and Vlachoudis;Vasilis and Vlastou;Rosa and Wallner;Anton and Woods;PhilipJohn and Wright;Tobias and Zugec;Petar and n TOF Collaboration
2023-01-01
Abstract
Background: The 14N(n, p) 14C reaction is of interest in neutron capturetherapy, where nitrogen-related dose is the main component due tolow-energy neutrons, and in astrophysics, where 14N acts as a neutronpoison in the s process. Several discrepancies remain between theexisting data obtained in partial energy ranges: thermal energy, keVregion, and resonance region. Purpose: We aim to measure the 14N(n, p)14C cross section from thermal to the resonance region in a singlemeasurement for the first time, including characterization of the firstresonances, and provide calculations of Maxwellian averaged crosssections (MACS). Method: We apply the time-of-flight technique atExperimental Area 2 (EAR-2) of the neutron time-of-flight (n\_TOF)facility at CERN. 10B(n, \& alpha;) 7Li and 235U(n, f ) reactions areused as references. Two detection systems are run simultaneously, one onbeam and another off beam. Resonances are described with the R-matrixcode SAMMY. Results: The cross section was measured from subthermalenergy to 800 keV, resolving the first two resonances (at 492.7 and 644keV). A thermal cross section was obtained (1.809 \& PLUSMN; 0.045 b)that is lower than the two most recent measurements by slightly morethan one standard deviation, but in line with the ENDF/B-VIII.0 andJEFF-3.3 evaluations. A 1/v energy dependence of the cross section wasconfirmed up to tens of keV neutron energy. The low energy tail of thefirst resonance at 492.7 keV is lower than suggested by evaluatedvalues, while the overall resonance strength agrees with evaluations.Conclusions: Our measurement has allowed determination of the 14N(n, p)cross section over a wide energy range for the first time. We haveobtained cross sections with high accuracy (2.5\%) from subthermalenergy to 800 keV and used these data to calculate the MACS for kT = 5to kT = 100 keV.
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.11769/590590
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